High-Energy X-Ray Compton Scattering Imaging of 18650-Type Lithium-Ion Battery Cell

Kosuke Suzuki; Ari-Pekka Honkanen; Naruki Tsuji; Kirsi Jalkanen; Jari Koskinen; Hideyuki Morimoto; Daisuke Hiramoto; Ayumu Terasaka; Hasnain Hafiz; Yoshiharu Sakurai; Mika Kanninen; Simo Huotari; Arun Bansil; Hiroshi Sakurai; Bernardo Barbiellini

doi:10.3390/condmat4030066

High-Energy X-Ray Compton Scattering Imaging of 18650-Type Lithium-Ion Battery Cell

Kosuke Suzuki, Ari-Pekka Honkanen, Naruki Tsuji, Kirsi Jalkanen, Jari Koskinen, Hideyuki Morimoto, Daisuke Hiramoto, Ayumu Terasaka, Hasnain Hafiz, Yoshiharu Sakurai, Mika Kanninen, Simo Huotari, Arun Bansil, Hiroshi Sakurai, Bernardo Barbiellini

Research output: Contribution to journal › Article › Scientific › peer-review

Abstract

High-energy synchrotron X-ray Compton scattering imaging was applied to a commercial 18650-type cell, which is a cylindrical lithium-ion battery in wide current use. By measuring the Compton scattering X-ray energy spectrum non-destructively, the lithiation state in both fresh and aged cells was obtained from two different regions of the cell, one near the outer casing and the other near the center of the cell. Our technique has the advantage that it can reveal the lithiation state with a micron-scale spatial resolution even in large cells. The present method enables us to monitor the operation of large-scale cells and can thus accelerate the development of advanced lithium-ion batteries.

Original language	English
Article number	66
Journal	Condensed matter
Volume	4
Issue number	3
Number of pages	8
ISSN	2410-3896
DOIs	https://doi.org/10.3390/condmat4030066
Publication status	Published - Sep 2019
MoE publication type	A1 Journal article-refereed

Fields of Science

114 Physical sciences

Access to Document

10.3390/condmat4030066Licence: CC BY

condensedmatter-04-00066Licence: CC BY

X-ray Laboratory
Simo Huotari (Manager)
Department of Physics
Facility/equipment: Research Laboratory

Cite this

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title = "High-Energy X-Ray Compton Scattering Imaging of 18650-Type Lithium-Ion Battery Cell",

abstract = "High-energy synchrotron X-ray Compton scattering imaging was applied to a commercial 18650-type cell, which is a cylindrical lithium-ion battery in wide current use. By measuring the Compton scattering X-ray energy spectrum non-destructively, the lithiation state in both fresh and aged cells was obtained from two different regions of the cell, one near the outer casing and the other near the center of the cell. Our technique has the advantage that it can reveal the lithiation state with a micron-scale spatial resolution even in large cells. The present method enables us to monitor the operation of large-scale cells and can thus accelerate the development of advanced lithium-ion batteries.",

keywords = "114 Physical sciences",

author = "Kosuke Suzuki and Ari-Pekka Honkanen and Naruki Tsuji and Kirsi Jalkanen and Jari Koskinen and Hideyuki Morimoto and Daisuke Hiramoto and Ayumu Terasaka and Hasnain Hafiz and Yoshiharu Sakurai and Mika Kanninen and Simo Huotari and Arun Bansil and Hiroshi Sakurai and Bernardo Barbiellini",

year = "2019",

month = sep,

doi = "10.3390/condmat4030066",

language = "English",

volume = "4",

journal = "Condensed matter",

issn = "2410-3896",

publisher = "MDPI AG",

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TY - JOUR

T1 - High-Energy X-Ray Compton Scattering Imaging of 18650-Type Lithium-Ion Battery Cell

AU - Suzuki, Kosuke

AU - Honkanen, Ari-Pekka

AU - Tsuji, Naruki

AU - Jalkanen, Kirsi

AU - Koskinen, Jari

AU - Morimoto, Hideyuki

AU - Hiramoto, Daisuke

AU - Terasaka, Ayumu

AU - Hafiz, Hasnain

AU - Sakurai, Yoshiharu

AU - Kanninen, Mika

AU - Huotari, Simo

AU - Bansil, Arun

AU - Sakurai, Hiroshi

AU - Barbiellini, Bernardo

PY - 2019/9

Y1 - 2019/9

N2 - High-energy synchrotron X-ray Compton scattering imaging was applied to a commercial 18650-type cell, which is a cylindrical lithium-ion battery in wide current use. By measuring the Compton scattering X-ray energy spectrum non-destructively, the lithiation state in both fresh and aged cells was obtained from two different regions of the cell, one near the outer casing and the other near the center of the cell. Our technique has the advantage that it can reveal the lithiation state with a micron-scale spatial resolution even in large cells. The present method enables us to monitor the operation of large-scale cells and can thus accelerate the development of advanced lithium-ion batteries.

AB - High-energy synchrotron X-ray Compton scattering imaging was applied to a commercial 18650-type cell, which is a cylindrical lithium-ion battery in wide current use. By measuring the Compton scattering X-ray energy spectrum non-destructively, the lithiation state in both fresh and aged cells was obtained from two different regions of the cell, one near the outer casing and the other near the center of the cell. Our technique has the advantage that it can reveal the lithiation state with a micron-scale spatial resolution even in large cells. The present method enables us to monitor the operation of large-scale cells and can thus accelerate the development of advanced lithium-ion batteries.

KW - 114 Physical sciences

U2 - 10.3390/condmat4030066

DO - 10.3390/condmat4030066

M3 - Article

VL - 4

JO - Condensed matter

JF - Condensed matter

SN - 2410-3896

IS - 3

M1 - 66

ER -

High-Energy X-Ray Compton Scattering Imaging of 18650-Type Lithium-Ion Battery Cell

Abstract

Fields of Science

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Equipment

X-ray Laboratory

Cite this