A study on the elongation of embedded Au nanoclusters in SiO2 by swift heavy ion irradiation using MD simulations

Aleksi Anssi Mikael Leino; Olli Heikki Pakarinen; Flyura Djurabekova; Kai Nordlund

doi:10.1016/j.nimb.2011.08.054

A study on the elongation of embedded Au nanoclusters in SiO2 by swift heavy ion irradiation using MD simulations

Aleksi Anssi Mikael Leino, Olli Heikki Pakarinen, Flyura Djurabekova, Kai Nordlund

Forskningsoutput: Tidskriftsbidrag › Konferensartikel › Vetenskaplig › Peer review

Sammanfattning

We have studied the elongation of Au nanoclusters embedded in amorphous SiO2 using MD simulations. The effect of swift heavy ions (SHI) was implemented using instantaneous energy deposition with a radial profile that was obtained from the inelastic thermal spike model. During the first impact on the cluster, the clusters (d = 9–11 nm) gained about 20% in length due to thermal stress within the cluster, which is released by a longitudinal flow of Au atoms to the ion track in silica. Our simulations also show that high temperatures at the track core lead to the formation of silica vapor, whose pressure may flatten the cluster.

Originalspråk	engelska
Tidskrift	Nuclear Instruments & Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms
Volym	282
Sidor (från-till)	76-80
Antal sidor	5
ISSN	0168-583X
DOI	https://doi.org/10.1016/j.nimb.2011.08.054
Status	Publicerad - 2012
MoE-publikationstyp	A4 Artikel i en konferenspublikation
Evenemang	Unknown host publication - , Holland Varaktighet: 1 jan. 1800 → …

Vetenskapsgrenar

114 Fysik

Åtkomst av dokument

10.1016/j.nimb.2011.08.054

Citera det här

@article{2abe04e0f2ee4e6c815b6b6d4e3a3930,

title = "A study on the elongation of embedded Au nanoclusters in SiO2 by swift heavy ion irradiation using MD simulations",

abstract = "We have studied the elongation of Au nanoclusters embedded in amorphous SiO2 using MD simulations. The effect of swift heavy ions (SHI) was implemented using instantaneous energy deposition with a radial profile that was obtained from the inelastic thermal spike model. During the first impact on the cluster, the clusters (d = 9–11 nm) gained about 20% in length due to thermal stress within the cluster, which is released by a longitudinal flow of Au atoms to the ion track in silica. Our simulations also show that high temperatures at the track core lead to the formation of silica vapor, whose pressure may flatten the cluster.",

keywords = "114 Physical sciences, molecular dynamics simulations, Ion-matter interactions, Elongation, NANOCLUSTERS, SILICA",

author = "Leino, {Aleksi Anssi Mikael} and Pakarinen, {Olli Heikki} and Flyura Djurabekova and Kai Nordlund",

note = " Volume: 282 Host publication title: E-MRS 2011 Proceedings ; Unknown host publication ; Conference date: 01-01-1800",

year = "2012",

doi = "10.1016/j.nimb.2011.08.054",

language = "English",

volume = "282",

pages = "76--80",

journal = "Nuclear Instruments & Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms",

issn = "0168-583X",

publisher = "Elsevier",

}

A study on the elongation of embedded Au nanoclusters in SiO2 by swift heavy ion irradiation using MD simulations. / Leino, Aleksi Anssi Mikael ; Pakarinen, Olli Heikki ; Djurabekova, Flyura et al.

I: Nuclear Instruments & Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms, Vol. 282, 2012, s. 76-80.

Forskningsoutput: Tidskriftsbidrag › Konferensartikel › Vetenskaplig › Peer review

TY - JOUR

T1 - A study on the elongation of embedded Au nanoclusters in SiO2 by swift heavy ion irradiation using MD simulations

AU - Leino, Aleksi Anssi Mikael

AU - Pakarinen, Olli Heikki

AU - Djurabekova, Flyura

AU - Nordlund, Kai

N1 - Volume: 282 Host publication title: E-MRS 2011 Proceedings

PY - 2012

Y1 - 2012

N2 - We have studied the elongation of Au nanoclusters embedded in amorphous SiO2 using MD simulations. The effect of swift heavy ions (SHI) was implemented using instantaneous energy deposition with a radial profile that was obtained from the inelastic thermal spike model. During the first impact on the cluster, the clusters (d = 9–11 nm) gained about 20% in length due to thermal stress within the cluster, which is released by a longitudinal flow of Au atoms to the ion track in silica. Our simulations also show that high temperatures at the track core lead to the formation of silica vapor, whose pressure may flatten the cluster.

AB - We have studied the elongation of Au nanoclusters embedded in amorphous SiO2 using MD simulations. The effect of swift heavy ions (SHI) was implemented using instantaneous energy deposition with a radial profile that was obtained from the inelastic thermal spike model. During the first impact on the cluster, the clusters (d = 9–11 nm) gained about 20% in length due to thermal stress within the cluster, which is released by a longitudinal flow of Au atoms to the ion track in silica. Our simulations also show that high temperatures at the track core lead to the formation of silica vapor, whose pressure may flatten the cluster.

KW - 114 Physical sciences

KW - molecular dynamics simulations

KW - Ion-matter interactions

KW - Elongation

KW - NANOCLUSTERS

KW - SILICA

U2 - 10.1016/j.nimb.2011.08.054

DO - 10.1016/j.nimb.2011.08.054

M3 - Conference article

VL - 282

SP - 76

EP - 80

JO - Nuclear Instruments & Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms

JF - Nuclear Instruments & Methods in Physics Research. Section B: Beam Interactions with Materials and Atoms

SN - 0168-583X

T2 - Unknown host publication

Y2 - 1 January 1800

ER -